Chemoenzymatic Cascades Combining Biocatalysis and Transition Metal Catalysis for Asymmetric Synthesis

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Abstract: The combination of catalytic methods provides multiple advantages in organic synthesis, allowing access to diverse organic molecules in a straightforward manner. Merging metal and enzyme catalysis is currently receiving great attention due to the possibility to assemble metal catalysis in C−C coupling, olefin metathesis, hydration and other reactions with the exquisite stereospecificity displayed by enzymes. Thus, this minireview is organized based on the action of the metal species (Pd, Ru, Au, Ir, Fe…) in combination with different enzymes. Special attention will be paid to the design of sequential processes and concurrent cascades, presenting solutions such as the use of surfactants or compartmentalization strategies for those cases where incompatibilities could hamper the overall process.

Location: Deutsche Nationalbibliothek Frankfurt am Main

Extent: Online-Ressource

Language: Englisch

Bibliographic citation: Chemoenzymatic Cascades Combining Biocatalysis and Transition Metal Catalysis for Asymmetric Synthesis ; day:28 ; month:02 ; year:2023 ; extent:16
Angewandte Chemie / International edition. International edition ; (28.02.2023) (gesamt 16)

Creator: González‐Granda, Sergio
Escot, Lorena
Lavandera, Iván
Gotor‐Fernández, Vicente

DOI: 10.1002/anie.202217713

URN: urn:nbn:de:101:1-2023022814363793290352

Rights: Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.

Last update: 14.08.2025, 10:44 AM CEST

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Associated

González‐Granda, Sergio
Escot, Lorena
Lavandera, Iván
Gotor‐Fernández, Vicente

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Chemoenzymatic Cascades Combining Biocatalysis and Transition Metal Catalysis for Asymmetric Synthesis

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Comprehensive asymmetric catalysis, 3

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Comprehensive asymmetric catalysis, 1

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Comprehensive asymmetric catalysis, 2

Comprehensive asymmetric catalysis, 2

Asymmetric Brønsted acid catalysis

Asymmetric Brønsted acid catalysis

Strategies in asymmetric catalysis

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Multi-step enzyme catalysis : biotransformations and chemoenzymatic synthesis

Multi-step enzyme catalysis : biotransformations and chemoenzymatic synthesis

Construction of Chemoenzymatic Linear Cascades for the Synthesis of Chiral Compounds

Construction of Chemoenzymatic Linear Cascades for the Synthesis of Chiral Compounds

Chemoenzymatic Dynamic Kinetic Asymmetric Transformations of β‐Hydroxyketones

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Interactive biocatalysis achieved by driving enzyme cascades inside a porous conducting material

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Bridging the gap between transition metal- and bio-catalysis via aqueous micellar catalysis

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Comprehensive asymmetric catalysis, 3

Comprehensive asymmetric catalysis, 1

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Asymmetric phase transfer catalysis

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Comprehensive asymmetric catalysis, 2

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Asymmetric Brønsted acid catalysis

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Strategies in asymmetric catalysis

Strategies in asymmetric catalysis

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