Elucidating ozone and PM<sub>2.5</sub> pollution in the Fenwei Plain reveals the co-benefits of controlling precursor gas emissions in winter haze

Abstract 2.5 or the O3 level-1 air quality standard, highlighting the severity of air pollution. Moreover, an increase in O3 pollution in the winter haze was also revealed, due to the constantly elevated reactive oxygenated volatile organic compounds (OVOCs), in particular formaldehyde, with an ozone formation potential of over 50 µ g m- 3 2. The abrupt decrease of NO2, as observed during the lockdown in 2020, provided real-world evidence of the control measures, targeting only NOx (70 % decrease on average), and were insufficient to reduce ozone pollution because reactive OVOCs remained constantly high in a volatile organic compound (VOC)-limited regime. Model simulation results showed that with NO2 reduction from 20 %–70 %, the self-reaction rate between peroxy radicals, a pathway for SOA formation, was intensified by up to 75 %, while the self-reaction rate was only reduced with a further reduction of VOCs of > 2.5 and O3 pollution can only be achieved through a more aggressive reduction of their precursor gases. This study elucidates the status of ozone and PM2.5 pollution in one of the most polluted regions in China, revealing a general trend of increasing secondary pollution, i.e., ozone and SOA in winter haze. Controlling precursor gas emissions is anticipated to curb both ozone and SOA formation, which will benefit not just the Fenwei Plain but also other regions in China.

Standort
Deutsche Nationalbibliothek Frankfurt am Main
Umfang
Online-Ressource
Sprache
Englisch

Erschienen in
Elucidating ozone and PM2.5 pollution in the Fenwei Plain reveals the co-benefits of controlling precursor gas emissions in winter haze ; volume:23 ; number:6 ; year:2023 ; pages:3595-3607 ; extent:13
Atmospheric chemistry and physics ; 23, Heft 6 (2023), 3595-3607 (gesamt 13)

Urheber
Lin, Chunshui
Huang, Ru-Jin
Zhong, Haobin
Duan, Jing
Wang, Zixi
Huang, Wei
Xu, Wei

DOI
10.5194/acp-23-3595-2023
URN
urn:nbn:de:101:1-2023033005260830894275
Rechteinformation
Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
Letzte Aktualisierung
14.08.2025, 10:56 MESZ

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Beteiligte

  • Lin, Chunshui
  • Huang, Ru-Jin
  • Zhong, Haobin
  • Duan, Jing
  • Wang, Zixi
  • Huang, Wei
  • Xu, Wei

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