Visualizing Dynamic Single Atom Catalysis
Abstract: Many industrial chemical processes, including for producing fuels, foods, pharmaceuticals, chemicals and environmental controls, employ heterogeneous solid state catalysts at elevated temperatures in gas or liquid environments. Dynamic reactions at the atomic level play a critical role in catalyst stability and functionality. In situ visualization and analysis of atomic‐scale processes in real time under controlled reaction environments can provide important insights into practical frameworks to improve catalytic processes and materials. This review focuses on innovative real time in situ electron microscopy (EM) methods, including recent progress in analytical in situ environmental (scanning) transmission EM (E (STEM), incorporating environmental scanning TEM (ESTEM) and environmental transmission EM (ETEM), with single atom resolution for visualizing and analysing dynamic single atom catalysis under controlled flowing gas reaction environments. ESTEM studies of single atom dynamics of reactions, and of sintering deactivation, contribute to a better‐informed understanding of the yield and stability of catalyst operations. Advances in in situ technologies, including gas and liquid sample holders, nanotomography, and higher voltages, as well as challenges and opportunities in tracking reacting atoms, are highlighted. The findings show that the understanding and application of fundamental processes in catalysis can be improved, with valuable economic, environmental, and societal benefits.
- Standort
-
Deutsche Nationalbibliothek Frankfurt am Main
- Umfang
-
Online-Ressource
- Sprache
-
Englisch
- Erschienen in
-
Visualizing Dynamic Single Atom Catalysis ; day:29 ; month:05 ; year:2024 ; extent:19
Advanced materials ; (29.05.2024) (gesamt 19)
- Urheber
-
Boyes, Edward D.
Gai, Pratibha L.
- DOI
-
10.1002/adma.202314121
- URN
-
urn:nbn:de:101:1-2405291429046.457326406285
- Rechteinformation
-
Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
- Letzte Aktualisierung
-
14.08.2025, 11:01 MESZ
Datenpartner
Deutsche Nationalbibliothek. Bei Fragen zum Objekt wenden Sie sich bitte an den Datenpartner.
Beteiligte
- Boyes, Edward D.
- Gai, Pratibha L.
Ähnliche Objekte (12)
Understanding the Dynamic Aggregation in Single‐Atom Catalysis
Modeling Single‐Atom Catalysis
Supported metal single atom catalysis
Single‐Atom Catalysis in Organic Synthesis
Single‐Atom Catalysis in Organic Synthesis
Dynamic chloride ion adsorption on single iridium atom boosts seawater oxidation catalysis
Single-Atom Catalysis: How Structure Influences Catalytic Performance
Isolating Single and Few Atoms for Enhanced Catalysis
Continuous Flow Single‐Atom Catalysis: A Viable Organic Process Technology? **
Polyoxometalate‐Single Atom Catalysts (POM‐SACs) in Energy Research and Catalysis
Solid Single‐Atom Catalysts in Tandem Catalysis: Lookout, Opportunities and Challenges
Visualizing dynamic data with heat triangles
Understanding the Dynamic Aggregation in Single‐Atom Catalysis
Modeling Single‐Atom Catalysis
Supported metal single atom catalysis
Single‐Atom Catalysis in Organic Synthesis
Single‐Atom Catalysis in Organic Synthesis
Dynamic chloride ion adsorption on single iridium atom boosts seawater oxidation catalysis
Single-Atom Catalysis: How Structure Influences Catalytic Performance
Isolating Single and Few Atoms for Enhanced Catalysis
Continuous Flow Single‐Atom Catalysis: A Viable Organic Process Technology? **
Polyoxometalate‐Single Atom Catalysts (POM‐SACs) in Energy Research and Catalysis
Solid Single‐Atom Catalysts in Tandem Catalysis: Lookout, Opportunities and Challenges
Visualizing dynamic data with heat triangles
Understanding the Dynamic Aggregation in Single‐Atom Catalysis
Modeling Single‐Atom Catalysis
Supported metal single atom catalysis
Single‐Atom Catalysis in Organic Synthesis
Single‐Atom Catalysis in Organic Synthesis
Dynamic chloride ion adsorption on single iridium atom boosts seawater oxidation catalysis
Single-Atom Catalysis: How Structure Influences Catalytic Performance
Isolating Single and Few Atoms for Enhanced Catalysis
Continuous Flow Single‐Atom Catalysis: A Viable Organic Process Technology? **
Polyoxometalate‐Single Atom Catalysts (POM‐SACs) in Energy Research and Catalysis
Solid Single‐Atom Catalysts in Tandem Catalysis: Lookout, Opportunities and Challenges