Wintertime subarctic new particle formation from Kola Peninsula sulfur emissions

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Abstract 2) emissions from the ore smelters are transported to wide areas, including Finnish Lapland. We performed investigations on concentrations of SO2, aerosol precursor vapours, aerosol and ion cluster size distributions together with chemical composition measurements of freshly formed clusters at the SMEAR I station in Finnish Lapland relatively close (∼ 2 from smelter emissions is converted to sulfuric acid (H2 SO4) in sufficient concentrations to drive new particle formation hundreds of kilometres downwind from the emission sources, even at very low solar radiation intensities. Observed new particle formation is primarily initiated by H2 SO4 –ammonia (negative-) ion-induced nucleation. Particle growth to cloud condensation nuclei (CCN) sizes was concluded to result from sulfuric acid condensation. However, air mass advection had a large role in modifying aerosol size distributions, and other growth mechanisms and condensation of other compounds cannot be fully excluded. Our results demonstrate the dominance of SO2 emissions in controlling wintertime aerosol and CCN concentrations in the subarctic region with a heavily polluting industry.

Location: Deutsche Nationalbibliothek Frankfurt am Main

Extent: Online-Ressource

Language: Englisch

Bibliographic citation: Wintertime subarctic new particle formation from Kola Peninsula sulfur emissions ; volume:21 ; number:23 ; year:2021 ; pages:17559-17576 ; extent:18
Atmospheric chemistry and physics ; 21, Heft 23 (2021), 17559-17576 (gesamt 18)

Creator: Sipilä, Mikko
Sarnela, Nina
Neitola, Kimmo
Laitinen, Totti
Kemppainen, Deniz
Beck, Lisa
Duplissy, Ella-Maria
Kuittinen, Salla
Lehmusjärvi, Tuuli
Lampilahti, Janne
Kerminen, Veli-Matti
Lehtipalo, Katrianne
Aalto, Pasi P.
Keronen, Petri
Siivola, Erkki
Rantala, Pekka A.
Worsnop, Douglas R.
Kulmala, Markku
Jokinen, Tuija
Petäjä, Tuukka

DOI: 10.5194/acp-21-17559-2021

URN: urn:nbn:de:101:1-2021120904341337064461

Rights: Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.

Last update: 15.08.2025, 7:29 AM CEST

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Sipilä, Mikko
Sarnela, Nina
Neitola, Kimmo
Laitinen, Totti
Kemppainen, Deniz
Beck, Lisa
Duplissy, Ella-Maria
Kuittinen, Salla
Lehmusjärvi, Tuuli
Lampilahti, Janne
Kerminen, Veli-Matti
Lehtipalo, Katrianne
Aalto, Pasi P.
Keronen, Petri
Siivola, Erkki
Rantala, Pekka A.
Worsnop, Douglas R.
Kulmala, Markku
Jokinen, Tuija
Petäjä, Tuukka

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Wintertime subarctic new particle formation from Kola Peninsula sulfur emissions

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Other Objects (12)

Wintertime sub-arctic new particle formation from Kola Peninsula sulphur emissions

Effect of ions on the measurement of sulfuric acid in the CLOUD experiment at CERN

Effect of ions on the measurement of sulphuric acid in the CLOUD experiment at CERN

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Measurement report: Long-term measurements of aerosol precursor concentrations in the Finnish sub-Arctic boreal forest

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