Microwave radiometer observations of the ozone diurnal cycle and its short-term variability over Switzerland

Abstract km): the GROund-based Millimeter-wave Ozone Spectrometer (GROMOS) in Bern (Institute of Applied Physics) and the Stratospheric Ozone MOnitoring RAdiometer (SOMORA) in Payerne (MeteoSwiss). Recently, their calibration and retrieval algorithms have been fully harmonized, and updated time series are now available since 2009. Using these harmonized ozone time series, we investigate and cross-validate the strato–mesospheric ozone diurnal cycle derived from the two instruments and compare it with various model-based datasets: the dedicated GEOS-GMI Diurnal Ozone Climatology (GDOC) based on the Goddard Earth Observing System (GEOS-5) general circulation model, the Belgian Assimilation System for Chemical ObsErvations (BASCOE) – a chemical transport model driven by ERA5 dynamics, and a set of free-running simulations from the Whole Atmosphere Community Climate Model (WACCM). Overall, the two instruments show very similar ozone diurnal cycles at all seasons and pressure levels, and the models compare well with each other. There is a good agreement between the models and the measurements at most seasons and pressure levels, and the largest discrepancies can be explained by the limited vertical resolution of the microwave radiometers. However, as in a similar study over Mauna Loa, some discrepancies remain near the stratopause, at the transition region between ozone daytime accumulation and depletion. We report similar delays in the onset of the modelled ozone diurnal depletion in the lower mesosphere. x) concentrations. However, we also find periods with an enhanced diurnal cycle that do not show much change in NOx and where other processes might be dominant (e.g. atmospheric tides). Given its importance, we believe that the short-term variability of the ozone diurnal cycle should be further investigated over the globe, for instance using the BASCOE model.

Location
Deutsche Nationalbibliothek Frankfurt am Main
Extent
Online-Ressource
Language
Englisch

Bibliographic citation
Microwave radiometer observations of the ozone diurnal cycle and its short-term variability over Switzerland ; volume:23 ; number:13 ; year:2023 ; pages:7321-7345 ; extent:25
Atmospheric chemistry and physics ; 23, Heft 13 (2023), 7321-7345 (gesamt 25)

Creator
Sauvageat, Eric
Hocke, Klemens
Maillard Barras, Eliane
Hou, Shengyi
Errera, Quentin
Haefele, Alexander
Murk, Axel

DOI
10.5194/acp-23-7321-2023
URN
urn:nbn:de:101:1-2023070604144236587042
Rights
Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
Last update
14.08.2025, 10:58 AM CEST

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Associated

  • Sauvageat, Eric
  • Hocke, Klemens
  • Maillard Barras, Eliane
  • Hou, Shengyi
  • Errera, Quentin
  • Haefele, Alexander
  • Murk, Axel

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