Transient Spin Injection Efficiencies at Ferromagnet–Metal Interfaces

Abstract: Spin injection across interfaces driven by ultrashort optical pulses on femtosecond timescales constitutes a new way to design spintronics applications. Targeted utilization of this phenomenon requires knowledge of the efficiency of non‐equilibrium spin injection. From a quantitative comparison of ab initio time‐dependent density functional theory and interface‐sensitive, time‐resolved non‐linear optical experiment, the spin injection efficiency (SIE) at the Co/Cu (001) interface is determined, and its microscopic origin, i.e., the influence of spin‐orbit coupling and the interface electronic structure, is discussed. Moreover, we theoretically predict that the SIE at ferromagnetic–metal interfaces can be optimized through laser pulse and materials parameters, namely the fluence, pulse duration, and substrate material.

Location
Deutsche Nationalbibliothek Frankfurt am Main
Extent
Online-Ressource
Language
Englisch

Bibliographic citation
Transient Spin Injection Efficiencies at Ferromagnet–Metal Interfaces ; day:19 ; month:10 ; year:2022 ; extent:9
Advanced materials interfaces ; (19.10.2022) (gesamt 9)

Creator
Elliott, Peter
Eschenlohr, Andrea
Chen, Jinghao
Shallcross, Sam
Bovensiepen, Uwe
Dewhurst, John Kay
Sharma, Sangeeta

DOI
10.1002/admi.202201233
URN
urn:nbn:de:101:1-2022102015183244093069
Rights
Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
Last update
15.08.2025, 7:29 AM CEST

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Associated

  • Elliott, Peter
  • Eschenlohr, Andrea
  • Chen, Jinghao
  • Shallcross, Sam
  • Bovensiepen, Uwe
  • Dewhurst, John Kay
  • Sharma, Sangeeta

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