Use of lidar aerosol extinction and backscatter coefficients to estimate cloud condensation nuclei (CCN) concentrations in the southeast Atlantic

Abstract S) greater than 0.25 % and dry ambient conditions above the stratocumulus deck, where relative humidity (RH) is less than 50 %. We find CCN–HSRL-2 Pearson correlation coefficients between 0.95–0.97 for different parts of the seasonal burning cycle that suggest fundamental similarities in biomass burning aerosol (BBA) microphysical properties. We find that ORACLES campaign-average values of in situ CCN and in situ extinction coefficients are qualitatively similar to those from other regions and aerosol types, demonstrating overall representativeness of our data set. We compute CCN–backscatter and CCN–extinction regressions that can be used to resolve vertical CCN concentrations across entire above-cloud lidar curtains. These lidar-derived CCN concentrations can be used to evaluate model performance, which we illustrate using an example CCN concentration curtain from the Weather Research and Forecasting Model coupled with physics packages from the Community Atmosphere Model version 5 (WRF-CAM5). These results demonstrate the utility of deriving vertically resolved CCN concentrations from lidar observations to expand the spatiotemporal coverage of limited or unavailable in situ observations.

Location
Deutsche Nationalbibliothek Frankfurt am Main
Extent
Online-Ressource
Language
Englisch

Bibliographic citation
Use of lidar aerosol extinction and backscatter coefficients to estimate cloud condensation nuclei (CCN) concentrations in the southeast Atlantic ; volume:16 ; number:7 ; year:2023 ; pages:2037-2054 ; extent:18
Atmospheric measurement techniques ; 16, Heft 7 (2023), 2037-2054 (gesamt 18)

Creator
Lenhardt, Emily D.
Gao, Lan
Redemann, Jens
Xu, Feng
Burton, Sharon P.
Cairns, Brian
Chang, Ian
Ferrare, Richard A.
Hostetler, Chris A.
Saide, Pablo E.
Howes, Calvin
Shinozuka, Yohei
Stamnes, Snorre
Kacarab, Mary
Dobracki, Amie
Wong, Jenny
Freitag, Steffen
Nenes, Athanasios

DOI
10.5194/amt-16-2037-2023
URN
urn:nbn:de:101:1-2023042005180646810693
Rights
Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
Last update
14.08.2025, 10:48 AM CEST

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Associated

  • Lenhardt, Emily D.
  • Gao, Lan
  • Redemann, Jens
  • Xu, Feng
  • Burton, Sharon P.
  • Cairns, Brian
  • Chang, Ian
  • Ferrare, Richard A.
  • Hostetler, Chris A.
  • Saide, Pablo E.
  • Howes, Calvin
  • Shinozuka, Yohei
  • Stamnes, Snorre
  • Kacarab, Mary
  • Dobracki, Amie
  • Wong, Jenny
  • Freitag, Steffen
  • Nenes, Athanasios

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