Symmetry‐Breaking Charge‐Transfer Chromophore Interactions Supported by Carbon Nanodots †
Abstract: Carbon dots (CDs) and their derivatives are useful platforms for studying electron‐donor/acceptor interactions and dynamics therein. Herein, we couple amorphous CDs with phthalocyanines (Pcs) that act as electron donors with a large extended π‐surface and intense absorption across the visible range of the solar spectrum. Investigations of the intercomponent interactions by means of steady‐state and pump‐probe transient absorption spectroscopy reveal symmetry‐breaking charge transfer/separation and recombination dynamics within pairs of phthalocyanines. The CDs facilitate the electronic interactions between the phthalocyanines. Thus, our findings suggest that CDs could be used to support electronic couplings in multichromophoric systems and further increase their applicability in organic electronics, photonics, and artificial photosynthesis.
- Standort
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Deutsche Nationalbibliothek Frankfurt am Main
- Umfang
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Online-Ressource
- Sprache
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Englisch
- Erschienen in
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Symmetry‐Breaking Charge‐Transfer Chromophore Interactions Supported by Carbon Nanodots † ; volume:132 ; number:31 ; year:2020 ; pages:12879-12884 ; extent:6
Angewandte Chemie ; 132, Heft 31 (2020), 12879-12884 (gesamt 6)
- Urheber
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Cacioppo, Michele
Scharl, Tobias
Đorđević, Luka
Cadranel, Alejandro
Arcudi, Francesca
Guldi, Dirk M.
Prato, Maurizio
- DOI
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10.1002/ange.202004638
- URN
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urn:nbn:de:101:1-2022053107395495142626
- Rechteinformation
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Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
- Letzte Aktualisierung
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15.08.2025, 07:29 MESZ
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Beteiligte
- Cacioppo, Michele
- Scharl, Tobias
- Đorđević, Luka
- Cadranel, Alejandro
- Arcudi, Francesca
- Guldi, Dirk M.
- Prato, Maurizio
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