Development of a Minimal Photosystem for Hydrogen Production in Inorganic Chemical Cells
Abstract: Inorganic chemical cells (iCHELLs) are compartment structures consisting of polyoxometalates (POMs) and cations, offering structured and confined reaction spaces bounded by membranes. We have constructed a system capable of efficient anisotropic and hierarchical photo‐induced electron transfer across the iCHELL membrane. Mimicking photosynthesis, our system uses proton gradients between the compartment and the bulk to drive efficient conversion of light into chemical energy, producing hydrogen upon irradiation. This illustrates the power of the iCHELL approach for catalysis, where the structure, compartmentalisation and variation in possible components could be utilised to approach a wide range of reactions.
- Location
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Deutsche Nationalbibliothek Frankfurt am Main
- Extent
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Online-Ressource
- Language
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Englisch
- Bibliographic citation
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Development of a Minimal Photosystem for Hydrogen Production in Inorganic Chemical Cells ; volume:57 ; number:40 ; year:2018 ; pages:13066-13070 ; extent:5
Angewandte Chemie / International edition. International edition ; 57, Heft 40 (2018), 13066-13070 (gesamt 5)
- Creator
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Nakanishi, Keita
Cooper, Geoffrey J. T.
Points, Laurie J.
Bloor, Leanne G.
Ohba, Masaaki
Cronin, Leroy
- DOI
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10.1002/anie.201805584
- URN
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urn:nbn:de:101:1-2022082209203657126732
- Rights
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Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
- Last update
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15.08.2025, 7:30 AM CEST
Data provider
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Associated
- Nakanishi, Keita
- Cooper, Geoffrey J. T.
- Points, Laurie J.
- Bloor, Leanne G.
- Ohba, Masaaki
- Cronin, Leroy
Other Objects (12)
Development of a Minimal Photosystem for Hydrogen Production in Inorganic Chemical Cells
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Bio-inorganic hybrid structures for direct electron transfer to photosystem I in photobioelectrodes
Biomimetic chiral hydrogen-bonded organic-inorganic frameworks
Ladungsrekombinationsreaktionen im Photosystem II
Industrial inorganic chemicals and products, Vol. 3.. Fertilizers to hydrogen
Superacids and acidic melts as inorganic chemical reaction media
DNA-Programmed Chemical Synthesis of Polymers and Inorganic Nanomaterials
Einzelmolekül-Spektroskopie am Photosystem I
Water oxidation in photosystem II
Energy transfer in Photosystem II
Structural studies on Photosystem II
Development of a Minimal Photosystem for Hydrogen Production in Inorganic Chemical Cells
Dynamic Hydrogen-Bonded Networks of Photosystem II
Bio-inorganic hybrid structures for direct electron transfer to photosystem I in photobioelectrodes
Biomimetic chiral hydrogen-bonded organic-inorganic frameworks
Ladungsrekombinationsreaktionen im Photosystem II
Industrial inorganic chemicals and products, Vol. 3.. Fertilizers to hydrogen
Superacids and acidic melts as inorganic chemical reaction media
DNA-Programmed Chemical Synthesis of Polymers and Inorganic Nanomaterials
Einzelmolekül-Spektroskopie am Photosystem I
Water oxidation in photosystem II
Energy transfer in Photosystem II
Structural studies on Photosystem II
Development of a Minimal Photosystem for Hydrogen Production in Inorganic Chemical Cells
Dynamic Hydrogen-Bonded Networks of Photosystem II
Bio-inorganic hybrid structures for direct electron transfer to photosystem I in photobioelectrodes
Biomimetic chiral hydrogen-bonded organic-inorganic frameworks
Ladungsrekombinationsreaktionen im Photosystem II
Industrial inorganic chemicals and products, Vol. 3.. Fertilizers to hydrogen
Superacids and acidic melts as inorganic chemical reaction media
DNA-Programmed Chemical Synthesis of Polymers and Inorganic Nanomaterials
Einzelmolekül-Spektroskopie am Photosystem I
Water oxidation in photosystem II
Energy transfer in Photosystem II