3D Highly Stretchable Liquid Metal/Elastomer Composites with Strain‐Enhanced Conductivity

Abstract: Current stretchable conductors, often composed of elastomeric composites infused with rigid conductive fillers, suffer from limited stretchability and durability, and declined conductivity with stretching. These limitations hinder their potential applications as essential components such as interconnects, sensors, and actuators in stretchable electronics and soft machines. In this context, an innovative elastomeric composite that incorporates a 3D network of liquid metal (LM), offering exceptional stretchability, durability, and conductivity, is introduced. The mechanics model elucidates how the interconnected 3DLM architecture imparts softness and stretchability to the composites, allowing them to withstand tensile strains of up to 500% without rupture. The relatively low surface‐to‐volume ratio of the 3DLM network limits the reforming of the oxide layer during cyclic stretch, thereby contributing to low permanent strain and enhanced durability. Additionally, the 3D architecture facilitates crack blunting and stress delocalization, elevating fracture resistance, while simultaneously establishing continuous conductive pathways that result in high conductivity. Notably, the conductivity of the 3DLM composite increases with strain during substantial stretching, highlighting its strain‐enhanced conductivity. In comparison to other LM‐based composites featuring 0D LM droplets, the 3DLM composite stands out with superior properties.

Location
Deutsche Nationalbibliothek Frankfurt am Main
Extent
Online-Ressource
Language
Englisch

Bibliographic citation
3D Highly Stretchable Liquid Metal/Elastomer Composites with Strain‐Enhanced Conductivity ; day:27 ; month:10 ; year:2023 ; extent:9
Advanced functional materials ; (27.10.2023) (gesamt 9)

Creator
Fang, Ruyue
Yao, Bin
Chen, Tianwu
Xu, Xinwei
Xue, Dingchuan
Hong, Wei
Wang, Hong
Wang, Qing
Zhang, Sulin

DOI
10.1002/adfm.202310225
URN
urn:nbn:de:101:1-2023102715341042642207
Rights
Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
Last update
14.08.2025, 10:48 AM CEST

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Associated

  • Fang, Ruyue
  • Yao, Bin
  • Chen, Tianwu
  • Xu, Xinwei
  • Xue, Dingchuan
  • Hong, Wei
  • Wang, Hong
  • Wang, Qing
  • Zhang, Sulin

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