Neutron Reflectometry of Lithium‐Based Secondary Batteries
The rapid advancement of integrated circuits and artificial intelligence has accelerated the proliferation of smart devices, driving the demand for high‐performance lithium‐based secondary batteries (LSBs). Despite notable technological advancements, LSBs continue to face significant challenges, particularly regarding cycle life, power density, specific capacity, and long‐term stability. To optimize these batteries, advanced analytical techniques are crucial for probing fundamental processes such as lithium‐ion migration, electrode material transformations, and solid electrolyte interphase evolution. While techniques such as scanning electron microscopy, transmission electron microscopy, and X‐ray reflectometry offer valuable insights into surface morphology and structural properties, their sensitivity limitations to lighter elements like lithium and hydrogen hinder comprehensive analysis. In contrast, neutron reflectometry (NR) provides a distinct advantage, offering nondestructive, lithium‐sensitive, and deeply penetrating insights into the internal dynamics of LSBs. In situ NR facilitates real‐time monitoring of structural transformations at the electrode/electrolyte interface and lithium distribution during cycling, while enabling the quantification of chemical composition under operational conditions. This review examines the advantages of NR over conventional techniques, evaluates its strengths and limitations, and surveys recent applications of NR in LSB research. The potential of NR in advancing the development of high‐performance LSB technologies is also discussed.
- Location
-
Deutsche Nationalbibliothek Frankfurt am Main
- Extent
-
Online-Ressource
- Language
-
Englisch
- Bibliographic citation
-
Neutron Reflectometry of Lithium‐Based Secondary Batteries ; day:25 ; month:12 ; year:2024 ; extent:19
Small structures ; (25.12.2024) (gesamt 19)
- Creator
-
Hu, Dengyan
Zhan, Xiaozhi
Wang, Xiaofei
Lin, Haibin
Gao, Lei
Tu, Haoran
Zhu, Jinlong
Zhu, Tao
Han, Songbai
- DOI
-
10.1002/sstr.202400542
- URN
-
urn:nbn:de:101:1-2412261308230.510341798511
- Rights
-
Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
- Last update
-
15.08.2025, 7:26 AM CEST
Data provider
Deutsche Nationalbibliothek. If you have any questions about the object, please contact the data provider.
Associated
- Hu, Dengyan
- Zhan, Xiaozhi
- Wang, Xiaofei
- Lin, Haibin
- Gao, Lei
- Tu, Haoran
- Zhu, Jinlong
- Zhu, Tao
- Han, Songbai
Other Objects (12)
Domestication of wild animals may provide a springboard for rapid variation of coronavirus
Correlation analysis of energy consumption, carbon emissions and economic growth
Equilibrium concepts in the large-household model
Unsteady porous-media flows
Existence and uniqueness of positive solutions for fractional differential equations
Dispute formatting: dispute transformation in case filing
An alternative error bound for linear complementarity problems involving BS $B^S}$-matrices
The crystal structure of samarium sulfate pentahydrate, Sm 2 (SO 4) 3 (H 2 O) 5
MRCT and CT in the diagnosis of pediatric disease imaging: assessing imaging performance and clinical effects
Direct links between hygroscopicity and mixing state of ambient aerosols: Estimating particle hygroscopicity from their single particle mass spectra
Doubly robust estimators for generalizing treatment effects on survival outcomes from randomized controlled trials to a target population
Frequency of intron loss correlates with processed pseudogene abundance: a novel strategy to test the reverse transcriptase model of intron loss
Domestication of wild animals may provide a springboard for rapid variation of coronavirus
Correlation analysis of energy consumption, carbon emissions and economic growth
Equilibrium concepts in the large-household model
Unsteady porous-media flows
Existence and uniqueness of positive solutions for fractional differential equations
Dispute formatting: dispute transformation in case filing
An alternative error bound for linear complementarity problems involving BS $B^S}$-matrices
The crystal structure of samarium sulfate pentahydrate, Sm 2 (SO 4) 3 (H 2 O) 5
MRCT and CT in the diagnosis of pediatric disease imaging: assessing imaging performance and clinical effects
Direct links between hygroscopicity and mixing state of ambient aerosols: Estimating particle hygroscopicity from their single particle mass spectra
Doubly robust estimators for generalizing treatment effects on survival outcomes from randomized controlled trials to a target population
Frequency of intron loss correlates with processed pseudogene abundance: a novel strategy to test the reverse transcriptase model of intron loss
Domestication of wild animals may provide a springboard for rapid variation of coronavirus
Correlation analysis of energy consumption, carbon emissions and economic growth
Equilibrium concepts in the large-household model
Unsteady porous-media flows
Existence and uniqueness of positive solutions for fractional differential equations
Dispute formatting: dispute transformation in case filing
An alternative error bound for linear complementarity problems involving BS $B^S}$-matrices
The crystal structure of samarium sulfate pentahydrate, Sm 2 (SO 4) 3 (H 2 O) 5
MRCT and CT in the diagnosis of pediatric disease imaging: assessing imaging performance and clinical effects
Direct links between hygroscopicity and mixing state of ambient aerosols: Estimating particle hygroscopicity from their single particle mass spectra
Doubly robust estimators for generalizing treatment effects on survival outcomes from randomized controlled trials to a target population