A Novel Domain‐Confined Growth Strategy for In Situ Controllable Fabrication of Individual Hollow Nanostructures
Abstract: The manipulation and tailoring of the structure and properties of semiconductor nanocrystals (NCs) is significant particularly for the design and fabrication of future nanodevices. Here, a novel domain‐confined growth strategy is reported for controllable fabrication of individual monocrystal hollow NCs (h‐NCs) in situ inside a transmission electron microscope, which enables the atomic scale monitoring of the entire reaction. During the process, the preformed carbon shells serve as nanoreaction cells for the formation of CdSeS h‐NCs. Electron beam (e‐beam) irradiation is demonstrated to be the key activation factor for the solid‐to‐hollow shape transformation. The formation of CdSeS hollow NCs is also found to be sensitive to the volume ratio of the CdSe/CdS NCs to the carbon shell and only those CdSe/CdS NCs with a volume ratio in the range 0.2–0.8 are successfully converted into hollow NCs. The method paves the way to potentially use an e‐beam for the in situ tailoring of individual semiconductor NCs targeted toward future nanodevice applications.
- Location
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Deutsche Nationalbibliothek Frankfurt am Main
- Extent
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Online-Ressource
- Language
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Englisch
- Bibliographic citation
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A Novel Domain‐Confined Growth Strategy for In Situ Controllable Fabrication of Individual Hollow Nanostructures ; volume:5 ; number:5 ; year:2018 ; extent:7
Advanced science ; 5, Heft 5 (2018) (gesamt 7)
- Creator
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Tang, Luping
He, Longbing
Zhang, Lei
Yu, Kaihao
Xu, Tao
Zhang, Qiubo
Dong, Hui
Zhu, Chao
Sun, Litao
- DOI
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10.1002/advs.201700213
- URN
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urn:nbn:de:101:1-2022091019181089712855
- Rights
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Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
- Last update
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15.08.2025, 7:21 AM CEST
Data provider
Deutsche Nationalbibliothek. If you have any questions about the object, please contact the data provider.
Associated
- Tang, Luping
- He, Longbing
- Zhang, Lei
- Yu, Kaihao
- Xu, Tao
- Zhang, Qiubo
- Dong, Hui
- Zhu, Chao
- Sun, Litao
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