Beyond-hot-spot absorption enhancement on top of terahertz nanotrenches

Abstract: Metallic nanogaps are being widely used for sensing applications, owing to their ability to confine and enhance electromagnetic field within the hot spots. Since the enhanced field does not confine itself perfectly within the gap, however, fringe fields well away from the gap are of potential use as well in real systems. Here, we extend the concept of near field absorption enhancement by quantitatively analyzing terahertz absorption behavior of water molecules outside the hot spots of sub-20 nm-wide, ∼100 μm-long nanotrenches. Contrary to point-gaps which show negligible field enhancement at distances larger than the gap width, our extended nanogap act as a line source, incorporating significant amount of absorption enhancement at much longer distances. We observe absorption enhancement factors of up to 3600 on top of a 5 nm-wide gap, and still well over 300 at 15 nm away. The finding is well supported by theoretical analyses including modal expansion calculations, Kirchhoff integral formalism and antenna theory. Our results provide means to quantitatively analyze light-matter interactions beyond the hot spot picture and enable application of nanogaps for sensitive surface analyses of various material systems.

Location
Deutsche Nationalbibliothek Frankfurt am Main
Extent
Online-Ressource
Language
Englisch

Bibliographic citation
Beyond-hot-spot absorption enhancement on top of terahertz nanotrenches ; volume:11 ; number:13 ; year:2022 ; pages:3159-3167 ; extent:9
Nanophotonics ; 11, Heft 13 (2022), 3159-3167 (gesamt 9)

Creator
Jeong, Jeeyoon
Kim, Dai-Sik
Park, Hyeong-Ryeol

DOI
10.1515/nanoph-2022-0214
URN
urn:nbn:de:101:1-2022120813082033062398
Rights
Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
Last update
15.08.2025, 7:32 AM CEST

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Associated

  • Jeong, Jeeyoon
  • Kim, Dai-Sik
  • Park, Hyeong-Ryeol

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