Polarization shaping of high-order harmonics in laser-aligned molecules

Abstract: The present work reports on the generation of short-pulse coherent extreme ultraviolet radiation of controlled polarization. The proposed strategy is based on high-order harmonics generated in pre-aligned molecules. Field-free molecular alignment produced by a short linearly-polarized infrared laser pulse is used to break the isotropy of a gas medium. Driving the aligned molecules by a circularly-polarized infrared pulse allows to transfer the anisotropy of the medium to the polarization of the generated harmonic light. The ellipticity of the latter is controlled by adjusting the angular distribution of the molecules at the time they interact with the driving pulse. Extreme ultraviolet radiation produced with high degree of ellipticity (close to circular) is demonstrated

Standort
Deutsche Nationalbibliothek Frankfurt am Main
Umfang
Online-Ressource
Sprache
Englisch
Anmerkungen
Scientific reports. - 6 (2016) , 39295, ISSN: 2045-2322

Ereignis
Veröffentlichung
(wo)
Freiburg
(wer)
Universität
(wann)
2019
Urheber
Skantzakis, Emmanouil
Chatziathanasiou, Stefanos
Carpeggiani, Paolo Antonio
Sansone, Giuseppe
Nayak, Arjun
Gray, D.
Tzallas, Paraskevas
Charalambidis, Dimitris
Hertz, Édouard
Faucher, Olivier

DOI
10.1038/srep39295
URN
urn:nbn:de:bsz:25-freidok-1441945
Rechteinformation
Kein Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
Letzte Aktualisierung
25.03.2025, 13:49 MEZ

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Entstanden

  • 2019

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