Side Chain Redistribution as a Strategy to Boost Organic Electrochemical Transistor Performance and Stability

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Abstract: A series of glycolated polythiophenes for use in organic electrochemical transistors (OECTs) is designed and synthesized, differing in the distribution of their ethylene glycol chains that are tethered to the conjugated backbone. While side chain redistribution does not have a significant impact on the optoelectronic properties of the polymers, this molecular engineering strategy strongly impacts the water uptake achieved in the polymers. By careful optimization of the water uptake in the polymer films, OECTs with unprecedented steady‐state performances in terms of [μC*] and current retentions up to 98% over 700 electrochemical switching cycles are developed.

Location: Deutsche Nationalbibliothek Frankfurt am Main

Extent: Online-Ressource

Language: Englisch

Bibliographic citation: Side Chain Redistribution as a Strategy to Boost Organic Electrochemical Transistor Performance and Stability ; volume:32 ; number:37 ; year:2020 ; extent:6
Advanced materials ; 32, Heft 37 (2020) (gesamt 6)

Creator: Moser, Maximilian
Hidalgo, Tania Cecilia
Surgailis, Jokubas
Gladisch, Johannes
Ghosh, Sarbani
Sheelamanthula, Rajendar
Thiburce, Quentin
Giovannitti, Alexander
Salleo, Alberto
Gasparini, Nicola
Wadsworth, Andrew
Zozoulenko, Igor
Berggren, Magnus
Stavrinidou, Eleni
Inal, Sahika
McCulloch, Iain

DOI: 10.1002/adma.202002748

URN: urn:nbn:de:101:1-2022062109261054552522

Rights: Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.

Last update: 15.08.2025, 7:26 AM CEST

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Moser, Maximilian
Hidalgo, Tania Cecilia
Surgailis, Jokubas
Gladisch, Johannes
Ghosh, Sarbani
Sheelamanthula, Rajendar
Thiburce, Quentin
Giovannitti, Alexander
Salleo, Alberto
Gasparini, Nicola
Wadsworth, Andrew
Zozoulenko, Igor
Berggren, Magnus
Stavrinidou, Eleni
Inal, Sahika
McCulloch, Iain

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Side Chain Redistribution as a Strategy to Boost Organic Electrochemical Transistor Performance and Stability

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Other Objects (12)

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Thermodynamics of organic electrochemical transistors

Processing of organic electrochemical transistors

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The combined influence of polythiophene side chains and electrolyte anions on organic electrochemical transistors

Interdigitated organic electrochemical transistors for biosensing

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Processing of organic electrochemical transistors

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Processing of organic electrochemical transistors

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