Unraveling the Mechanism of the Light‐Triggered Synaptic Plasticity in Organic Photoelectric Synaptic Transistors

Abstract: Light‐triggered synaptic plasticity (LTSP) induced by electron trapping in organic photoelectric synaptic transistors (OPSTs) offers potential prospects in neuromorphic wearable artificial intelligence. However, a consistent and universal comprehend for LTSP behaviors especially on oxygen effect in OPSTs is still a critical challenge hindering their practical applications. A mechanism on strong dependency between the oxygen‐induced and polar‐group electron trapping in OPSTs, is successfully unveiled in this study for the first time. And the interaction between the oxygen and polar dielectric interface can be enhanced by properly modulating the specific surface area of thin‐film semiconductors. This effectively binds the oxygen near conducting channel and further improves the trapping efficiency for photogenerated electrons, undergoing the time‐dependent photocurrent generation and subsequent prolonged decay, forming the typical LTSP behaviors. These experimental demonstrations differ from previous reports and therefore may contribute an innovative perspective in the design of functional layers for high‐performance OPST devices.

Standort
Deutsche Nationalbibliothek Frankfurt am Main
Umfang
Online-Ressource
Sprache
Englisch

Erschienen in
Unraveling the Mechanism of the Light‐Triggered Synaptic Plasticity in Organic Photoelectric Synaptic Transistors ; day:24 ; month:01 ; year:2024 ; extent:8
Advanced electronic materials ; (24.01.2024) (gesamt 8)

Urheber
Zhang, Cong
Zhang, Mingxin
Lin, Fengyuan
Zhao, Guodong
Wei, Zhipeng
Ni, Yanping
Li, Juntong
Yu, Hongyan
Zhao, Xiaoli
Tong, Yanhong
Tang, Qingxin
Liu, Yichun

DOI
10.1002/aelm.202300878
URN
urn:nbn:de:101:1-2024012514155623904866
Rechteinformation
Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
Letzte Aktualisierung
15.08.2025, 07:29 MESZ

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Beteiligte

  • Zhang, Cong
  • Zhang, Mingxin
  • Lin, Fengyuan
  • Zhao, Guodong
  • Wei, Zhipeng
  • Ni, Yanping
  • Li, Juntong
  • Yu, Hongyan
  • Zhao, Xiaoli
  • Tong, Yanhong
  • Tang, Qingxin
  • Liu, Yichun

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