Anisotropic 2D van der Waals Magnets Hosting 1D Spin Chains
Abstract: The exploration of 1D magnetism, frequently portrayed as spin chains, constitutes an actively pursued research field that illuminates fundamental principles in many‐body problems and applications in magnonics and spintronics. The inherent reduction in dimensionality often leads to robust spin fluctuations, impacting magnetic ordering and resulting in novel magnetic phenomena. Here, structural, magnetic, and optical properties of highly anisotropic 2D van der Waals antiferromagnets that uniquely host spin chains are explored. First‐principle calculations reveal that the weakest interaction is interchain, leading to essentially 1D magnetic behavior in each layer. With the additional degree of freedom arising from its anisotropic structure, the structure is engineered by alloying, varying the 1D spin chain lengths using electron beam irradiation, or twisting for localized patterning, and spin textures are calculated, predicting robust stability of the antiferromagnetic ordering. Comparing with other spin chain magnets, these materials are anticipated to bring fresh perspectives on harvesting low‐dimensional magnetism.
- Location
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Deutsche Nationalbibliothek Frankfurt am Main
- Extent
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Online-Ressource
- Language
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Englisch
- Bibliographic citation
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Anisotropic 2D van der Waals Magnets Hosting 1D Spin Chains ; day:03 ; month:06 ; year:2024 ; extent:9
Advanced materials ; (03.06.2024) (gesamt 9)
- Creator
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Park, Eugene
Philbin, John P.
Chi, Hang
Sanchez, Joshua J.
Occhialini, Connor
Varnavides, Georgios
Curtis, Jonathan B.
Song, Zhigang
Klein, Julian
Thomsen, Joachim D.
Han, Myung‐Geun
Foucher, Alexandre C.
Mosina, Kseniia
Kumawat, Deepika
Gonzalez‐Yepez, N.
Zhu, Yimei
Sofer, Zdeněk
Comin, Riccardo
Moodera, Jagadeesh S.
Narang, Prineha
Ross, Frances M.
- DOI
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10.1002/adma.202401534
- URN
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urn:nbn:de:101:1-2406031420043.538983360722
- Rights
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Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
- Last update
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14.08.2025, 10:57 AM CEST
Data provider
Deutsche Nationalbibliothek. If you have any questions about the object, please contact the data provider.
Associated
- Park, Eugene
- Philbin, John P.
- Chi, Hang
- Sanchez, Joshua J.
- Occhialini, Connor
- Varnavides, Georgios
- Curtis, Jonathan B.
- Song, Zhigang
- Klein, Julian
- Thomsen, Joachim D.
- Han, Myung‐Geun
- Foucher, Alexandre C.
- Mosina, Kseniia
- Kumawat, Deepika
- Gonzalez‐Yepez, N.
- Zhu, Yimei
- Sofer, Zdeněk
- Comin, Riccardo
- Moodera, Jagadeesh S.
- Narang, Prineha
- Ross, Frances M.