Enhanced Photoluminescence of Cesium Lead Halide Perovskites by Quasi‐3D Photonic Crystals

Abstract: Cesium lead halide perovskite nanocrystals have emerged as one of the most promising candidates for manufacturing portable lasers and light sources. In order to harness and exploit their photoluminescence more effectively, the nanocrystals are often accompanied by a photonic scheme that improves light emission. In this work, one introduces a quasi‐3D photonic crystal composed of a 2D‐grating on top of a distributed Bragg reflector (DBR) that provides a greater photoluminescence enhancement than the isolated architectures alone. The quasi‐3D photonic crystals support both Rayleigh‐Wood anomalies and guided modes that populate the photonic bandgap of the Bragg mirror, all of them capable of enhancing the outcoupling of light from the emitting layer. In order to demonstrate the benefits of the quasi‐3D system, one prepares 2D‐gratings, DBRs, and quasi‐3D photonic crystals covered with metal halide perovskite nanocrystals and studies the photoluminescence enhancement produced in each case. Interestingly, the quasi‐3D structure exhibits a photoluminescence enhancement of 16 times and an increase in spontaneous emission rate, greatly exceeding the values observed for the separate components.

Standort
Deutsche Nationalbibliothek Frankfurt am Main
Umfang
Online-Ressource
Sprache
Englisch

Erschienen in
Enhanced Photoluminescence of Cesium Lead Halide Perovskites by Quasi‐3D Photonic Crystals ; day:03 ; month:12 ; year:2021 ; extent:9
Advanced optical materials ; (03.12.2021) (gesamt 9)

Urheber
Carreño, José Mendoza
Passarelli, Nicolás
Otero, Clara
Polavarapu, Lakshminarayana
Pérez, Luis A.
Reparaz, Juan Sebastián
Alonso, María Isabel
Mihi, Agustin

DOI
10.1002/adom.202101324
URN
urn:nbn:de:101:1-2021120714392475041084
Rechteinformation
Open Access; Der Zugriff auf das Objekt ist unbeschränkt möglich.
Letzte Aktualisierung
15.08.2025, 07:23 MESZ

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